This study used a design experiment that instructs children on how to approach each letter to investigate typography design methodologies and manual techniques. Since children are still in the early stages of learning and the content they are exposed to is of great significance, the topic of children's education is always one that the entire community is intensely interested in discussing. According to researchers, typography is a popular medium and expressive technique in technology development, and art education is important for improving human communication. Typography with illustration may also help children achieve a clear sense of each letter's collocation by means of expression, recognition, and understanding through children's cognitive development by adding handcraft activities to each letter's characters. To approach new design considerations in typography and typeface experimentation, the current research analyses children's learning materials to consider their learning obstacles. Using an innovative design approach method in children's learning materials, this study demonstrates how children's drive to learn may be inspired and encouraged by a more engaging learning environment, leading to improved learning outcomes. Using paper-folding graphic visualization can also help kids understand the shape of each letter.